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Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Maekawa, Fujio; Meigo, Shinichiro
Proceedings of 14th International Particle Accelerator Conference (IPAC 23) (Internet), p.1591 - 1593, 2023/05
The Japan Atomic Energy Agency (JAEA) is designing a 30 MW continuous wave (cw) superconducting proton linear accelerator (linac) for the Accelerator Driven System (ADS) proposal. The JAEA-ADS linacs ion source must provide a proton beam over 20 mA with an energy of 35 keV and a normalized rms emittance of less than 0.1 
mm mrad. As the extraction system determines the beam properties and quality, systematic optimizations on the geometry and input values of the extraction system design were conducted using the AXCEL-INP 2-D simulation program to satisfy the goal requirements. This work describes the extraction system design and reports the beam dynamics results of the first study for the proton source of the JAEA-ADS linac.
Takei, Hayanori
Journal of Nuclear Science and Technology, 14 Pages, 2023/00
Times Cited Count：0 Percentile：0.08(Nuclear Science & Technology)In the proton linear accelerator (linac), the proton beam is unexpectedly interrupted due to the electrical discharge originating from the radio frequency, failure of the device/equipment, or other factors. Do these beam trips occur randomly? Conventionally, it has been implicitly assumed that beam trips occur randomly. In this study, we investigated whether beam trips in the linac of the Japan Proton Accelerator Research Complex (J-PARC) occur randomly to estimate the beam trip frequency in a superconducting proton linac for an accelerator-driven nuclear transmutation system. First, the J-PARC linac was classified into five subsystems. Then, the reliability function for the operation time in each subsystem was obtained using the Kaplan--Meier estimation, a reliability engineering methods. Using this reliability function, the randomness of beam trips was examined. Analysis of five-year operational data for five subsystems of the J-PARC linac showed that beam trips occurred randomly in some subsystems. However, beam trips did not occur randomly in many subsystems of the proton linac, including the ion source and the acceleration cavity, the primary subsystems of the proton linac.
Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro; Pyeon, C. H.*; Yamamoto, Akio*; Endo, Tomohiro*
Nuclear Science and Engineering, 20 Pages, 2023/00
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)In this study, we have demonstrated that data assimilation using lead and bismuth sample reactivities measured in the Kyoto University Critical Assembly A-core can successfully reduce the uncertainty of the coolant void reactivity in accelerator-driven systems derived from inelastic-scattering cross-sections of lead and bismuth. We re-evaluated and highlighted the experimental uncertainties and correlations of the sample reactivities for the data assimilation formula. We used the MCNP6.2 code to evaluate the sample reactivities and their uncertainties, and performed data assimilation using the reactor analysis code system MARBLE. The high-sensitivity coefficients of the sample reactivities to lead and bismuth allowed us to reduce the cross-section-induced uncertainty of the void reactivity of the accelerator-driven system from 6.3% to 4.8%, achieving a provisional target accuracy of 5% in this study. Furthermore, we demonstrated that the uncertainties arising from other dominant factors, such as minor actinides and steel, can be effectively reduced by using integral experimental data sets for the unified cross-section dataset ADJ2017.
Maekawa, Fujio
JAEA-Conf 2022-001, p.7 - 13, 2022/11
The partitioning and transmutation (P-T) technology has promising potential for volume reduction and mitigation of degree of harmfulness of high-level radioactive waste. JAEA is developing the P-T technology combined with accelerator driven systems (ADS). One of critical issues affecting the feasibility of ADS is the proton beam window (PBW) which functions as a boundary between the accelerator and the sub-critical reactor core. The PBW is damaged by a high-intensity proton beam and spallation neutrons produced in the target, and also by flowing high-temperature liquid lead bismuth eutectic alloy which is corrosive to steel materials. To study the materials damage under the ADS environment, J-PARC is proposing a plan of proton irradiation facility which equips with a liquid lead-bismuth spallation target bombarded by a 400 MeV - 250 kW proton beam. The facility is also open for versatile purposes such as soft error testing of semi-conductor devises, RI production, materials irradiation for fission and fusion reactors, and so on. Application to nuclear data research with using the proton beam and spallation neutrons is also one of such versatile purposes, and we welcome unique ideas from the nuclear data community.
Katano, Ryota; Yamamoto, Akio*; Endo, Tomohiro*
Nuclear Science and Engineering, 196(10), p.1194 - 1208, 2022/10
Times Cited Count：1 Percentile：29.26(Nuclear Science & Technology)In this study, we propose the ROM-Lasso method that enables efficient evaluation of sensitivity coefficients of neutronics parameters to cross-sections. In the proposed method, a vector of sensitivity coefficients is expanded by subspace bases, so-called Active Subspace (AS) based on the idea of Reduced Order Modeling (ROM). Then, the expansion coefficients are evaluated by the Lasso linear regression between cross-sections and neutronics parameters obtained by the random sampling. The proposed method can be applied in the case where the adjoint method is difficult to be applied since the proposed method uses only forward calculations. In addition, AS is an effective subspace that can expand the vector of sensitivity coefficients with the lower number of dimension. Thus, the number of unknows is reduced from the original number of input parameters and the calculation cost is dramatically improved compared to the Lasso regression without AS. In this paper, we conducted ADS burnup calculations as a verification. We have shown how AS bases are obtained and the applicability of the proposed method.
Ariyoshi, Gen; Obayashi, Hironari; Sasa, Toshinobu
Journal of Nuclear Science and Technology, 59(9), p.1071 - 1088, 2022/09
Times Cited Count：1 Percentile：29.26(Nuclear Science & Technology)Electromagnetic induction method is one of the effective techniques for local velocity measurement in heavy liquid metals. Ricou and Vives' probe and Von Weissenfluh's probe are famous instrumentations using a permanent magnet. However, sensitivity and measurement volume of the probes show unexpected variation since demagnetization of the magnet is occurred by temperature increase up to the Curie temperature. In this study, electromagnetic probe incorporating a miniature electromagnet was newly developed to overcome such unexpected variation. The diameter and the length of the sensor was 6 mm and 155 mm, respectively. The sensitivity and the measurement volume of the probe were assessed by measurement of local velocity of flowing mercury in a square channel. To clarify the validity for the measured velocity profiles, numerical velocity profiles were calculated and compared with experiment. And the validity for the measured velocity profiles were confirmed by calculated result.
Sr analysis of environmental samples by ion-laser interaction mass spectrometryHonda, Maki; Martschini, M.*; Marchhart, O.*; Priller, A.*; Steier, P.*; Golser, R.*; Sato, Tetsuya; Tsukada, Kazuaki; Sakaguchi, Aya*
Analytical Methods, 14(28), p.2732 - 2738, 2022/07
Times Cited Count：2 Percentile：43.32(Chemistry, Analytical)The sensitive Sr analysis with accelerator mass spectrometry (AMS) was developed for the advances of environmental radiology. One advantage of AMS is the ability to analyze various environmental samples with Sr/
Sr atomic ratios of 10
in a simple chemical separation. Three different IAEA samples with known Sr concentrations (moss-soil, animal bone, Syrian soil: 1 g each) were analyzed to assess the validity of the chemical separation and the AMS measurement. The Sr measurements were conducted on the AMS system combined with the Ion Laser InterAction MasSpectrometry (ILIAMS) setup at the University of Vienna, which has excellent isobaric separation performance. The isobaric interference of Zr in the Sr AMS was first removed by chemical separation. The separation factor of Zr in two-step column chromatography with Sr resin and anion exchange resin was 10
. The Zr remaining in the sample was removed by ILIAMS effectively. This simple chemical separation achieved a limit of detection 
0.1 mBq in the Sr AMS, which is lower than typical 
-ray detection. The agreement between AMS measurements and nominal values for the Sr concentrations of IAEA samples indicated that the new highly-sensitive Sr analysis in the environmental samples with AMS is reliable even for high matrix samples of soil and bone.
Maekawa, Fujio
Purazuma, Kaku Yugo Gakkai-Shi, 98(5), p.201 - 205, 2022/05
The nuclear transmutation technology is a powerful solution to the "nuclear waste" problem that accompanies nuclear power generation. The Accelerator Driven System (ADS), which combines a high-intensity accelerator and a subcritical core, is a promising tool for nuclear transmutation. In this paper, we will explain the significance and principle of nuclear transmutation by ADS, design examples of ADS, partitioning and transmutation technology and its effects, required performance of high-intensity accelerators, overseas trends, etc.
Maekawa, Fujio; Takei, Hayanori
Purazuma, Kaku Yugo Gakkai-Shi, 98(5), p.206 - 210, 2022/05
In developing an accelerator-driven nuclear transmutation system (ADS), it is necessary to solve technical issues related to proton beams, such as the development of materials that can withstand high-intensity proton beams and the characterization of subcritical cores driven by proton beams. Therefore, at the high-intensity proton accelerator facility J-PARC, a transmutation experimental facility that actually conducts various tests using a high-intensity proton beam is being planned. This paper introduces the outline and future direction of the transmutation experimental facility.
Sasa, Toshinobu
Purazuma, Kaku Yugo Gakkai-Shi, 98(5), p.211 - 215, 2022/05
Lead-bismuth eutectic (LBE) alloy is promising as a spallation target for next-generation reactor coolants and accelerator drive systems (ADS) due to its nuclear and chemical properties. LBE is a heavy metal, and it has good properties both as a spallation target and as a coolant for nuclear transmutation systems of long-lived radioactive nuclei. On the other hand, to improve compatibility with structural materials is one of the major issues in its utilization. The latest research results such as high-temperature operation of LBE and oxygen concentration control to ensure corrosion resistance with the aim of early commercialization of nuclear conversion technology by ADS is introduced.
Meigo, Shinichiro; Nakano, Keita; Iwamoto, Hiroki
Purazuma, Kaku Yugo Gakkai-Shi, 98(5), p.216 - 221, 2022/05
For the realization of accelerator-driven transmutation systems (ADS) and the construction of the ADS target test facility (TEF-T) at J-PARC, it is necessary to study the proton beam handling technology and neutronics for protons in the GeV energy region. Accordingly, the Nuclear Transmutation Division of J-PARC has studied these issues with using J-PARC's accelerator facilities, and so on. This paper introduces these topics.
Yb for producing 
Lu with high radionuclide purity by Yb(
)LuNagai, Yasuki*; Kawabata, Masako*; Hashimoto, Shintaro; Tsukada, Kazuaki; Hashimoto, Kazuyuki*; Motoishi, Shoji*; Saeki, Hideya*; Motomura, Arata*; Minato, Futoshi; Ito, Masatoshi*
Journal of the Physical Society of Japan, 91(4), p.044201_1 - 044201_10, 2022/04
Times Cited Count：2 Percentile：44.06(Physics, Multidisciplinary)Recently, Lu is considered as one of the most important medical RIs for treating neuroendocrine tumors. A plan to produce Lu with high purity by using enriched Yb samples with irradiation of deuteron beams in accelerators has been discussed. However, since the other Yb isotopes contained in the Yb sample interacts with deuterons, Lu isotopes other than Lu are produced as impurities. Since the purity of Lu is important for medical use, a method to evaluate the impurity of Lu has been required. In this study, we proposed a new method to estimate production yields of each Lu isotopes in Yb samples with arbitrary isotopic compositions by using excitation functions of Yb()Lu reactions and the particle transport calculation code PHITS. The method plays an important role in discussing the isotopic composition of enriched samples to produce high-purity Lu using accelerators.
Obayashi, Hironari; Yamaki, Kenichi*; Yoshimoto, Hidemitsu*; Kita, Satoshi*; Wan, T.*; Sasa, Toshinobu
JAEA-Technology 2021-035, 66 Pages, 2022/03
JAEA-Technology-2021-035.pdf:4.26MB
Construction of Transmutation Experimental Facility (TEF) is under planning in Japan Proton Accelerator Research Complex (J-PARC) program to promote R&Ds on realization of transmutation technology by an accelerator driven system (ADS). As a facility of TEF, ADS Target Test Facility (TEF-T) will provide a spallation target to study target technology and perform post irradiation examination (PIE) of candidate materials of ADS. In ADS, lead-bismuth eutectic (LBE) alloy is used as a spallation target material and a core coolant. As is well known, LBE has corrosive to structural materials hence each component of the target system should provide compatibility with LBE. In addition, instrumentations for LBE are restricted by the target operation condition such as high temperature and irradiation environment. The devices for LBE have been developed individually to achieve the LBE target system. "Integrated Multi-functional MOckup for TEF-T Real-scale TArget Loop, IMMORTAL" was fabricated as a mock-up test loop of the target for the purpose of the integration testing of individually developed devices. This report describes an overview of IMMORTAL and the design of the installed devices.
Nakano, Keita; Iwamoto, Hiroki; Nishihara, Kenji; Meigo, Shinichiro; Sugawara, Takanori; Iwamoto, Yosuke; Takeshita, Hayato*; Maekawa, Fujio
JAEA-Research 2021-018, 41 Pages, 2022/03
JAEA-Research-2021-018.pdf:2.93MB
Neutronic analysis of beam window of the Accelerator-Driven System (ADS) proposed by Japan Atomic Energy Agency (JAEA) has been conducted using PHITS and DCHAIN-PHITS codes. We investigate gas production of hydrogen and helium isotopes in the beam window, displacement per atom of beam window material, and heat generation in the beam window. In addition, distributions of produced nuclides, heat density, and activity are derived. It was found that at the maximum 12500 appm H production, 1800 appm He production, and damage of 62.1 DPA occurred in the beam window by the ADS operation. On the other hand, the maximum heat generation in the beam window was 374 W/cm
. In the analysis of LBE, 
Bi and 
Po were found to be the dominant nuclides in decay heat and radioactivity. Furthermore, the heat generation in the LBE by the proton beam was maximum around 5 cm downstream of the beam window, which was 945 W/cm.
Nakano, Keita; Matsuda, Hiroki*; Meigo, Shinichiro; Iwamoto, Hiroki; Takeshita, Hayato*; Maekawa, Fujio
JAEA-Research 2021-014, 25 Pages, 2022/03
JAEA-Research-2021-014.pdf:2.1MB
For the development of accelerator-driven transmutation system (ADS), measurement of nuclide production cross-sections in proton-induced reactions on 
Be, C, 
Al, 
Sc, and V have been performed. The measured data are compared with the calculations by the latest nuclear reaction models and with the nuclear data library to investigate the reproducibilities.
Hain, K.*; Martschini, M.*; G
lce, F.*; Honda, Maki; Lachner, J.*; Kern, M.*; Pitters, J.*; Quinto, F.*; Sakaguchi, Aya*; Steier, P.*; et al.
Frontiers in Marine Science (Internet), 9, p.837515_1 - 837515_17, 2022/03
Times Cited Count：12 Percentile：95.34(Environmental Sciences)Recent major advances in accelerator mass spectrometry (AMS) at the Vienna Environmental Research Accelerator (VERA) regarding detection efficiency and isobar suppression have opened possibilities for the analysis of additional long-lived radionuclides at ultra-low environmental concentrations. These radionuclides, including 
U, 
Cs, 
Tc and Sr, will become important for oceanographic tracer application due to their generally conservative behavior in ocean water. In particular, the isotope ratios U/
U and 
Cs/Cs have proven to be powerful fingerprints for emission source identification as they are not affected by elemental fractionation. Improved detection efficiencies allowed us to analyze all major long-lived actinides, i.e. U, 
Np, 
Pu, 
Am as well as the very rare U, in the same 10 L water samples of an exemplary depth profile from the northwest Pacific Ocean. Especially for Sr analysis, our new approach has already been validated for selected reference materials (e.g. IAEA-A-12) and is ready for application in oceanographic studies. We estimate that a sample volume of only (1-3) L ocean water is sufficient for Sr as well as Cs analysis, respectively.
Katano, Ryota
Journal of Nuclear Science and Technology, 59(3), p.368 - 381, 2022/03
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)We propose a subcriticality determination methodology to be applied during fuel loading of an accelerator-driven system (ADS). In this methodology, subcriticality is determined via the area ratio method (via the proton accelerator) in the first step and by the neutron source multiplication method (through the spontaneous fission neutrons of minor actinides) in subsequent steps; then, the number of fuel assemblies to be loaded in the next step is predicted. We performed a numerical simulation of the proposed methodology, and the estimated subcriticalities agreed well with those obtained by eigenvalue calculations. We also conducted an uncertainty assessment of the proposed methodology and deduced a value of 1000 pcm for the 
uncertainty. The proposed methodology can be a candidate for practical subcriticality monitoring for ADS.
Teshigawara, Makoto; Nakamura, Mitsutaka; Kinsho, Michikazu; Soyama, Kazuhiko
JAEA-Technology 2021-022, 208 Pages, 2022/02
JAEA-Technology-2021-022.pdf:14.28MB
The Materials and Life science experimental Facility (MLF) is an accelerator driven pulsed spallation neutron and muon source with a 1 MW proton beam. The construction began in 2004, and we started beam operation in 2008. Although problems such as exudation of cooling water from the target container have occurred, as of April 2021, the proton beam power has reached up to 700 kW gradually, and stable operation is being performed. In recent years, the operation experience of the rated 1 MW has been steadily accumulated. Several issues such as the durability of the target container have been revealed according to the increase in the operation time. Aiming at making a further improvement of MLF, we summarized the current status of achievements for the design values, such as accelerator technology (LINAC and RCS), neutron and muon source technology, beam transportation of these particles, detection technology, and neutron and muon instruments. Based on the analysis of the current status, we tried to extract improvement points for upgrade of MLF. Through these works, we will raise new proposals that promote the upgrade of MLF, attracting young people. We would like to lead to the further success of researchers and engineers who will lead the next generation.
Nakanoya, Takamitsu; Kamiya, Junichiro; Yoshimoto, Masahiro; Takayanagi, Tomohiro; Tani, Norio; Kotoku, Hirofumi*; Horino, Koki*; Yanagibashi, Toru*; Takeda, Osamu*; Yamamoto, Kazami
JAEA-Technology 2021-019, 105 Pages, 2021/11
JAEA-Technology-2021-019.pdf:10.25MB
Since a user operation startup, the 3 GeV synchrotron accelerator (Rapid-Cycling Synchrotron: RCS) gradually reinforced the beam power. As a result, the surface dose rate of the apparatus located at the beam injection area of the RCS, such as the magnet, vacuum chambers, beam monitors, etc., increases year by year. The beam injection area has many apparatuses which required manual maintenance, so reducing worker's dose is a serious issue. To solve this problem, we have organized a task force for the installation of the shield. The task force has aimed to optimize the structure of the radiation shield, construct the installation procedure with due consideration of the worker's dose suppression. As the examination result of the shield design, we have decided to adopt removal shielding that could be installed quickly and easily when needed. We carried out shield installation work during the 2020 summer maintenance period. The renewal work required to install the shielding has been carried out in a under high-dose environment. For this reason, reducing the dose of workers was an important issue. So, we carefully prepared the work plan and work procedure in advance. During the work period, we implemented various dose reduction measures and managed individual dose carefully. As a result, the dose of all workers could be kept below the predetermined management value. We had installed removal shielding at the beam injection area in the 2020 summer maintenance period. We confirmed that this shield can contribute to the reduction of the dose during work near the beam injection area. It was a large-scale work to occupy the beam injection area during almost of the summer maintenance period. However, it is considered very meaningful for dose suppression in future maintenance works.
Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*
Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.850 - 854, 2021/10
no abstracts in English
